Concentrations and Water Mass Transport of Legacy POPs in the Arctic Ocean
Document Type
Article
Date of Original Version
12-16-2018
Abstract
The Arctic Ocean is known to be contaminated by various persistent organic pollutants (POPs). The Fram Strait, the only deepwater passage to the Arctic Ocean (from the Atlantic Ocean), represents an unquantified gateway for POPs fluxes into and out of the Arctic. Polyethylene passive samplers were deployed in vertical profiles in the Fram Strait and in air and surface water in the Canadian Archipelago to determine the concentrations, profiles, and mass fluxes of dissolved polychlorinated biphenyls (PCBs) and organochlorine pesticides. In the Fram Strait, higher concentrations of ΣPCBs (1.3–3.6 pg/L) and dichlorodiphenyltrichloroethanes (ΣDDTs, 5.2–9.1 pg/L) were observed in the deepwater masses (below 1,000 m), similar to nutrient-like vertical profiles. There was net southward transport of hexachlorobenzene and hexachlorocyclohexanes (ΣHCHs) of 0.70 and 14 Mg/year but a net northward transport of ΣPCBs at 0.16 Mg/year through the Fram Strait.
Publication Title, e.g., Journal
Geophysical Research Letters
Volume
45
Issue
23
Citation/Publisher Attribution
Ma, Yuxin, Dave A. Adelman, Eduard Bauerfeind, Ana Cabrerizo, Carrie A. McDonough, Derek Muir, Thomas Soltwedel, Caoxin Sun, Charlotte C. Wagner, Elsie M. Sunderland, and Rainer Lohmann. "Concentrations and Water Mass Transport of Legacy POPs in the Arctic Ocean." Geophysical Research Letters 45, 23 (2018). doi: 10.1029/2018GL078759.