Title

Dispersion of the resonant nonlinear optical susceptibility obtained with femtosecond time-domain coherent anti-Stokes Raman scattering

Document Type

Article

Date of Original Version

11-15-2013

Abstract

We propose and experimentally demonstrate a method that is capable of resolving both real and imaginary parts of third-order nonlinearity (X (3)) in the vicinity of Raman resonances. Dispersion of X (3) can be obtained from a medium probed within microscopic volumes with a spectral resolution of better than 0.10 cm-1. © 2013 Optical Society of America.

Publication Title

Optics Letters

Volume

38

Issue

22

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